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Spatiotemporal spectroscopic characterization of plasmas induced by non-orthogonal laser ablation

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D0AN01996H.pdf (1.841Mb)
Date
2020-11-23
Author
Képeš, Erik
Gornushkin, Igor
Pořízka, Pavel
Kaiser, Jozef
Altmetrics
10.1039/D0AN01996H
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Abstract
Ablation geometry significantly affects the plasma parameters and the consequent spectroscopic observations in laser-induced breakdown spectroscopy. Nevertheless, plasmas induced by laser ablation under inclined incidence angles are studied to a significantly lesser extent compared to plasmas induced by standard orthogonal ablation. However, inclined ablation is prominent in stand-off applications, such as the Curiosity Mars rover, where the orthogonality of the ablation laser pulse cannot be always secured. Thus, in this work, we characterize non-orthogonal ablation plasmas by applying plasma imaging, tomography, and spectral measurements. We confirm earlier observations according to which non-orthogonal ablation leads to a laser-induced plasma that consists of two distinct parts: one expanding primarily along the incident laser pulse and one expanding along the normal of the sample surface. Moreover, we confirm that the former emits mainly continuum radiation, while the latter emits mainly sample-specific characteristic radiation. We further investigate and compare the homogeneity of the plasmas and report that inclined ablation affects principally the ionic emissivity of laser-induced plasmas. Overall, our results imply that the decreased fluence resulting from inclined angle ablation and the resulting inhomogeneities of the plasmas must be considered for quantitative LIBS employing non- orthogonal ablation.
Keywords
laser-induced plasma, laser-induced breakdown spectroscopy, non-orthogonal ablation, plasma tomography, Radon reconstruction
Persistent identifier
http://hdl.handle.net/11012/196476
Document type
Peer reviewed
Document version
Postprint
Source
ANALYST. 2020, vol. 146, issue 3, p. 920-929.
https://pubs.rsc.org/en/content/articlepdf/2021/AN/D0AN01996H
DOI
10.1039/D0AN01996H
Collections
  • Ústav fyzikálního inženýrství [102]
  • Pokročilé instrumentace a metody pro charakterizace materiálů [35]
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